Synthesis and characterization of high-sensitivity Dy,Eu co-doped CaSO4 thermoluminescent phosphor using coprecipitation technique.

In this work, (99 - x)CaSO4 -Dy2 O3 -xEu2 O3 , (where x = 0, 0.05, 0.1, 0.2, 0.3, 0.4, 0.5) thermoluminescence phosphors were prepared using a coprecipitation method. The thermoluminescence (TL) dosimetry (TLD) characteristics such as TL sensitivity, dose-response, minimum detectable dose, thermal fading, and the effect of sunlight on the prepared phosphors were investigated. The obtained results indicated that the most sensitive phosphor was obtained at x = 0.05. Large thermal fading of 6% after 1 h and 26% after 24 h from irradiation followed by 71% after 1 month with no additional fading was observed within a time frame exceeding 2 months throughout the remaining duration of the investigation, which also spanned over 2 months. Despite the phosphor's high fading rate, the relative sensitivity of the prepared samples was ~90% compared with TLD-100. The marked effect of day sunlight was also determined. High dose-response within the low-dose range from 0.01 to 5 Gy was observed. The obtained results suggested that the synthesized phosphor is well suited for applications involving radiation biology and radiotherapy dosimetry.

A Fiber-Optical Dosimetry Sensor for Gamma-Ray Irradiation Measurement in Biological Applications.

In this paper, we propose a novel fiber-optical dosimetry sensor for radiation measurement in biological applications. A two-dimensional (2D) fiber-optical dosimeter (FOD) for radiation measurement is considered. The sensors are arranged as a 2D array in a tailored holder. This FOD targets accurate industrial and medical applications which seek more tolerant radiation dosimeters. In this paper, the FOD sensors are subjected to gamma-ray radiation facilities from the 137Cs gamma-ray irradiator type for low doses and 60Co gamma-ray irradiator for high doses. For better evaluation of radiation effects on the FOD sample, the measurements are performed using eight sensors (hollow cylinder shape) with two samples in each dose. The sensors were measured before and after each irradiation. To the author's knowledge, the measurements of FOD transplanted inside animals are presented for the first time in this paper. A 2D simulation program has been implemented for numerical simulation based on the attenuation factors from the absorbed dose inside the in vivo models. A comparison between the FOD and the standard thermo-luminescence detector is presented based on the test of in vivo animal models. The results indicate that the proposed FOD sensor is more stable and has higher sensitivity.

Uncertainty of LiF thermoluminescence at low dose levels: Experimental results.

The LiF:Mg,Ti (TLD-100) thermoluminescence (TL) detectors are widely used in many dosimetric applications, particularly in personal dosimetry area. In the present study, the uncertainty of TLD-100 measurements at the low dose levels has been assessed for different TL readout analysis methods. The criteria used to evaluate the minimum measurable dose (MMD) have been also investigated. It has been found that between-sample variations and the precision of the TL measurements were the significant uncertainty components. However, the precision of the measurement is critically dependent on the TL readout analysis and background (BG) subtraction methods. The estimation of the MMD based on the 3σBG approach may lead to inaccurate measurements. On the other hand, a new criterion for evaluating the MMD based on the signal-to-noise ratio and can be evaluated from the glow-curve deconvolution analysis has been established. It has been shown that the implementation of this criterion ensures acceptable levels for both the precision and trueness of TL measurements.

Thermoluminescence glow curve deconvolution and kinetic parameter determination of samarium-doped lithium borosilicate glass.

Thermoluminescence glow curves of gamma-irradiated samarium-doped lithium borosilicate glass were investigated. The number of overlapping peaks was determined using the repeated initial rise method. The glow curves were deconvoluted into four overlapping peaks. The trapping parameters such as activation energy E, frequency factor (s), and kinetic order (b) for each peak were determined. The obtained results indicated that the lithium borosilicate glass doped with samarium had four electron trap levels with the average activation energies of 0.82, 1.01, 1.21, and 1.31 eV. Thermal fading analysis of the individual peaks based on the deconvolution data was performed. The obtained results showed high thermal fading of the first peak, but high thermal stability of the second and third peaks compared with the other peaks. These results could be used to explain some observed properties such as high thermal fading and light sensitivity for this thermoluminescent material. Moreover, the obtained results may be helpful in minimizing fading corrections in dosimetric applications.

Thermoluminescence characteristics of lithium borosilicate glass doped with Sm2 O3.

Lithium borosilicate glass composite (SiO2 -Li2 CO3 -H3 BO3 ) doped with various concentrations of Sm2 O3 (0-0.7 mole %) was prepared using the melt quenching method. The investigated thermoluminescence (TL) characteristics of the prepared system revealed that the highest TL response was obtained for this glass composite at 0.05 mol% Sm2 O3 . In this study, the 0.05 mol% Sm2 O3 -doped lithium borosilicate glass composite was subjected to detailed dosimetric investigation in terms of its annealing condition, dose-response, and minimum detectable dose. The reproducibility of the response, thermal characteristics, and optical fading were also studied. The obtained results showed that the prepared glass composite had a linear dose-response over the wide gamma dose range 2Gy to 2 kGy, as well as reasonable thermal fading and excellent reproducibility. These attributes render the composite under investigation promising for utilization in radiation detection.